The 128Mb card running 1000MHz video ram should outperform the 256Mb card running 900MHz video RAM. If you are after pure speed, then that's the deciding factor.
If, on the other hand, you are going to be insistent on running the highest graphical details you can possibly put on screen, regardless of whether or not it causes slowdows, then the extra video RAM would help with the massive texture calculations.
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Grandad
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since Mar 2004